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Stochastic model and intermediate asymptotics for charge transport in organic semiconductors

Stodtmann, Sven

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Abstract

A molecular scale model for charge transport in organic semiconductors based on quantum chemistry is presented. It is formulated as a stochastic model on the integer lattice in three dimensions. The model is treated with probabilistic methods, which allow to prove a continuous scaling limit, especially suited for intermediate regiemes, i.e. low temperatures, large energetic disorder and small devices. The scaling limit is connected to a certain integro-differential equation. Both, the microscopic model and the scaling limit are computationally studied and it is demonstrated that the proposed model can explain dispersive effects in thin film organic semiconductor devices.

Document type: Dissertation
Supervisor: Jäger, Prof. Dr. Dr. hc. mult Willi
Date of thesis defense: 13 February 2015
Date Deposited: 09 Mar 2015 10:50
Date: 2015
Faculties / Institutes: The Faculty of Mathematics and Computer Science > Institut für Mathematik
DDC-classification: 500 Natural sciences and mathematics
510 Mathematics
Controlled Keywords: Organischer Halbleiter, Stochastischer Prozess, Logarithmische Normalverteilung, Coarse graining, Gebrochene Analysis
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