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Attosecond dynamics of dipole-coupled doubly excited states in helium

Hu, Shuyuan

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Abstract

Within this work, electron dynamics in atoms are experimentally and numerically investigated on their natural attosecond time scales. To access these dynamics, ultrashort and moderately intense few-cycle laser pulses are superposed with attosecond pulsed radiation in the extreme-ultraviolet spectral region In particular, a bound two-electron wave packet in helium on attosecond time scales was experimentally observed. A novel experiment is presented to simultaneously measure resonant photoabsorption spectra of laser-coupled doubly excited states in helium and the streaked photoelectron spectra. It provides the advantage of obtaining an absolute calibration of the time-delay zero for absorption spectra, where delay-dependent phase information is extracted.

Document type: Dissertation
Supervisor: Pfeifer, Prof. Dr. Thomas
Place of Publication: Heidelberg
Date of thesis defense: 13 December 2023
Date Deposited: 14 Feb 2024 13:57
Date: 2024
Faculties / Institutes: The Faculty of Physics and Astronomy > Dekanat der Fakultät für Physik und Astronomie
Controlled Keywords: attosecond physics, attosecond streaking, time-resolved spectroscopy
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