title: Quantum control of x-ray spectra creator: Cavaletto, Stefano Michele subject: ddc-530 subject: 530 Physics description: The direct and optical control of x-ray transitions is studied theoretically by investigating the spectra of resonance fluorescence and absorption. The work is motivated by the rapid advances in x-ray science, enabling the application of quantum-control schemes at short wavelengths. In a two-level system we study Rabi oscillations of atomic inner-shell electrons, induced by intense x-ray pulses and competing with Auger decay, and their signature in the spectrum of resonance fluorescence. Subsequently, optical manipulation of x-ray transitions is examined, by employing an optical frequency comb coupling nearby excited levels to control their spontaneous decay. First, narrow-bandwidth x rays are adopted, giving rise to the periodic shaping of the atomic dynamic variables and the imprinting of a comb onto the x-ray resonance fluorescence spectrum. A more realistic model for an immediate experimental implementation is then provided, by developing a scheme to imprint a comb onto the absorption spectrum of an ultrashort x-ray pulse. An experimental realization of the predicted comb structures is anticipated to transfer the accuracy of optical frequency combs into the x-ray regime. date: 2013 type: Dissertation type: info:eu-repo/semantics/doctoralThesis type: NonPeerReviewed format: application/pdf identifier: https://archiv.ub.uni-heidelberg.de/volltextserverhttps://archiv.ub.uni-heidelberg.de/volltextserver/15982/1/Cavaletto-Thesis.pdf identifier: DOI:10.11588/heidok.00015982 identifier: urn:nbn:de:bsz:16-heidok-159820 identifier: Cavaletto, Stefano Michele (2013) Quantum control of x-ray spectra. [Dissertation] relation: https://archiv.ub.uni-heidelberg.de/volltextserver/15982/ rights: info:eu-repo/semantics/openAccess rights: http://archiv.ub.uni-heidelberg.de/volltextserver/help/license_urhg.html language: eng