%0 Generic %A Oelmann, Jan-Hendrik %C Heidelberg %D 2023 %F heidok:33225 %K Velocity-map imaging, Multipass cell, XUV frequency comb %R 10.11588/heidok.00033225 %T Highly nonlinear light-matter interaction using cavity-enhanced frequency combs %U https://archiv.ub.uni-heidelberg.de/volltextserver/33225/ %X Cavity-enhanced frequency combs are a powerful tool for studying highly nonlinear light-matter interactions, such as multiphoton ionization (MPI) and high-harmonic generation (HHG), with promising prospects for precision spectroscopy beyond the optical spectral range. In this work, a metrology-capable extreme ultraviolet (XUV) frequency comb is produced by transferring a near-infrared comb at 1039 nm to the XUV, using intra-cavity HHG. Intensities of ∼1E14 W/cm² are reached in the cavity focus, producing XUV radiation up to 42 eV (30 nm) and tens of microwatts of outcoupled power. A high-pressure closed-loop noble gas recycling and compression system enables long-term measurements. Additionally, a novel polarization-insensitive cavity with an integrated velocity-map imaging spectrometer was developed. 3D photoelectron angular distributions from xenon MPI are tomographically reconstructed, revealing resonant Rydberg states during ionization. Furthermore, polarization-shaped pulse pairs with a variable time delay are provided for pump-probe experiments. Intense femtosecond standing waves, produced by counter-propagating pulses colliding at the focus, are probed at the nanometer scale using photoemission from a nano-tip. The coherence of the frequency comb is imprinted on the photoelectrons, allowing future precision measurements with coherent matter waves. This work broadens the scope of cavity-enhanced frequency combs and enables strong-field studies at 100 MHz repetition rate.