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Quenching of Molecular Photodissociation by Interatomic Coulombic Decay

Kopelke, Sören

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Abstract

The impact of Interatomic Coulombic Decay (ICD) on the photoinduced dynamics in the first four vibrational levels of the first Rydberg state of CO in CO-Mg clusters is investigated. A method for calculating the required ICD widths is introduced. The method is tested by calculations of ICD widths of outer-valence excited states in NeAr, HCN-Mg and inner-valence excited states in NeMg.

Translation of abstract (German)

Der Einfluss des Interatomic Coulombic Decay (ICD) auf die Kerndynamik in den ersten vier Vibrations-Zuständen des ersten Rydberg-Zustandes in CO-Mg wird quantitativ untersucht. Eine Methode zur Berechnung der dazu benötigten ICD-Breiten wird eingeführt. Die Methode wird anhand von Berechnungen der ICD-Breiten von Anregungen in der äußeren Valenc in NeAr, HCN-Mg und in der inneren Valenz in NeMg getestet.

Item Type: Dissertation
Supervisor: Cederbaum, Prof. Dr. Lorenz S.
Date of thesis defense: 7. December 2011
Date Deposited: 15. Dec 2011 08:31
Date: 2011
Faculties / Institutes: Fakultät für Chemie und Geowissenschaften > Institute of Physical Chemistry
Subjects: 530 Physics
Uncontrolled Keywords: Interatomic , Coulombic , Decay , Quenching , Photodissociation
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